Effect of plasmonic Au nanoparticles on IR luminescence of Ag2S quantum dots
Abstract
Luminescent manifestations of the interaction of Ag2S quantum dots (QDs) with Au nanorods (NRs) depending on the overlap degree of the corresponding luminescence bands and plasmon resonance peaks have been experimentally established. Under spectral resonance conditions, the possibility of controlling the intensity of QDs luminescence by changing the interaction with Au NRs by varying the distance between the components of the plasmon-exciton mixture has been demonstrated. In turn it determines the influence of the near-field of metal nanoparticles on photoprocesses in Ag2S QDs.
The detuning of the spectral resonance due to the change in the Au QDs length leads to the asymmetry of the spectral contour of the Ag2S QDs luminescence band, which may be due to the manifestation of the Fano effect during plasmonexciton interaction, taking into account the inhomogeneous broadening of the corresponding bands
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